Hi mpls.
Awesome question this cloud sync dance can get tricky, any way...
First off, big yes u can absolutely use SharePoint Migration Tool (SPMT) with your Azure File Share as the source, since your files are already tiered to Azure (thanks to that ALOM attribute), SPMT will see them directly in the cloud. No need to pull them back down to on-prem how cool is that?
Microsoft-specific solution Fire up a VM in Azure (make sure it's same region as your file share!), install SPMT there, and point it to your Azure File Share path. You'll get way faster transfers since everything's already in the cloud neighborhood. https://docs.microsoft.com/en-us/azure/storage/files/storage-sync-files-planning.
Check your Azure File Share throughput at https://portal.azure.com. Sometimes upgrading the performance tier gives you that extra oomph. This trick works for other cloud storage tools too!
Before you dive in, take a peek at your Azure File Sync cloud tiering settings at https://docs.microsoft.com/en-us/azure/storage/files/storage-sync-cloud-tiering. Might want to tweak the policy so fewer files play hide-and-seek during migration.
always do a test run first! SPMT's trial migration feature at https://docs.microsoft.com/en-us/sharepointmigration/how-to-use-the-sharepoint-migration-tool will save you from permission nightmares later ))
Let us know how it goes
Best regards,
Alex
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